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Redox reactions of iron and manganese oxides in complex systems

Jianzhi Huang, Huichun Zhang

Frontiers of Environmental Science & Engineering 2020, Volume 14, Issue 5, doi: 10.1007/s11783-020-1255-8

Abstract: • Mechanisms of redox reactions of Fe- and Mn-oxides were discussed. • Oxidative reactions of Mn- andFe-oxides in complex systems were reviewed. • Reductive reaction of Fe(II)/iron oxides in complex systemsConspectus Redox reactions of Fe- and Mn-oxides play important roles in the fate and transformationreductive reactivity of Fe(II)/iron oxides in complex model systems toward contaminant degradation.such as Al, Si and Ti oxides on the redox reactivity of the systems are briefly summarized.

Keywords： Iron oxides     manganese oxides     reduction     oxidation     complex systems     reaction kinetics and mechanisms    

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Modified iron-molybdate catalysts with various metal oxides by a mechanochemical method: enhanced formaldehyde

Xue Liu, Lingtao Kong, Shengtao Xu, Chaofan Liu, Fengyun Ma

Frontiers of Chemical Science and Engineering 2021, Volume 15, Issue 5,   Pages 1099-1110 doi: 10.1007/s11705-020-2008-8

Abstract: A mechanochemical method was employed to prepare modified iron molybdate catalysts with various metalThe physicochemical properties of the iron molybdate catalysts were characterized, and their performancesIron molybdate catalysts doped with Co(NO ) ·6H O and Al(NO ) ·9H O resulted in high HCHO yields.MoO sublimation rate could be important factors enhancing the HCHO yield in reactions catalyzed with iron

Keywords： iron molybdate catalyst     metal oxides     methanol to formaldehyde     Co/Mo ratio     formaldehyde yield    

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Catalytic ozonation performance and surface property of supported Fe

Zhendong YANG, Aihua LV, Yulun NIE, Chun HU

Frontiers of Environmental Science & Engineering 2013, Volume 7, Issue 3,   Pages 451-456 doi: 10.1007/s11783-013-0509-0

Abstract: Fe O was supported on mesoporous Al O or SiO (50 wt.%) using an incipient wetness impregnation method, and Fe O /Al O exhibited higher catalytic efficiency for the degradation of 2,4-dichlorophenoxyacetic acid and -chlorobenzoic acid aqueous solution with ozone. The effect and morphology of supported Fe O on catalytic ozonation performance were investigated based on the characterization results of X-ray diffraction, X-ray photoelectron spectroscopy, BET analysis and Fourier transform infrared spectroscopy. The results indicated that the physical and chemical properties of the catalyst supports especially their Lewis acid sites had a significant influence on the catalytic activity. In comparison with SiO , more Lewis acid sites existed on the surface of Al O , resulting in higher catalytic ozonation activity. During the reaction process, no significant Fe ions release was observed. Moreover, Fe O /Al O exhibited stable structure and activity after successive cyclic experiments. The results indicated that the catalyst is a promising ozonation catalyst with magnetic separation in drinking water treatment.

Keywords： heterogeneous catalytic ozonation     iron oxides     supports     surface Lewis acid sites    

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Catalytic combustion of volatile organic compounds using perovskite oxides catalysts—a review

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 11,   Pages 1649-1676 doi: 10.1007/s11705-023-2324-x

Abstract: Next, the characteristics and catalytic performance of perovskite oxides as catalysts for VOC removalThe challenges and the prospects regarding the design of perovskite oxides catalysts for the catalytic

Keywords： perovskite oxides     volatile organic compounds     catalytic combustion     reaction mechanism    

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Multivalent manganese oxides with high electrocatalytic activity for oxygen reduction reaction

Xiangfeng Peng, Zhenhai Wang, Zhao Wang, Yunxiang Pan

Frontiers of Chemical Science and Engineering 2018, Volume 12, Issue 4,   Pages 790-797 doi: 10.1007/s11705-018-1706-y

Abstract: A noble-metal-free catalyst based on both Mn O and MnO was prepared by using the dielectric barrier discharge technique at moderate temperature. The prepared catalyst shows a higher electrocatalytic activity towards the oxygen reduction reaction than the catalyst prepared by using the traditional calcination process. The enhanced activity could be due to the coexistence of manganese ions with different valences, the higher oxygen adsorption capacity, and the suppressed aggregation of the catalyst nanoparticles at moderate temperature. The present work would open a new way to prepare low-cost and noble-metal-free catalysts at moderate temperature for more efficient electrocatalysis.

Keywords： oxygen reduction reaction     manganese oxides     mixed valences of manganese     oxygen adsorption     dielectric barrier    

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The role of manganese oxides in the activation of peroxymonosulfate (PMS)

Jianzhi Huang, Huichun Zhang

Frontiers of Environmental Science & Engineering 2019, Volume 13, Issue 5, doi: 10.1007/s11783-019-1158-8

Abstract: Manganese oxides (MnOx) have been demonstrated to be effective materials to activate Oxone (i.e., PMS

Keywords： Peroxymonosulfate     Manganese oxides     Catalyst     Oxidant    

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Review on research and application of mesoporous transitional metal oxides in water treatment

Minghao SUI, Lei SHE

Frontiers of Environmental Science & Engineering 2013, Volume 7, Issue 6,   Pages 795-802 doi: 10.1007/s11783-013-0521-4

Abstract: This paper reviews the application of mesoporous transitional metal oxides in water treatment on basisMesoporous transitional metal oxides are characterized by their intrinsic features, such as a high surface

Keywords： mesoporous materials     transitional metal oxides     catalysis     adsorption     water treatment    

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randomized, controlled, open label non-inferiority trial of intravenous ferric carboxymaltose versus ironsucrose in patients with iron deficiency anemia in China

Frontiers of Medicine doi: 10.1007/s11684-023-1001-2

Abstract: Iron deficiency (ID) and ID anemia (IDA) pose significant public health concerns in China.Although iron sucrose (IS) treatment is well-established in the country, ferric carboxymaltose (FCM)conducted at multiple sites in China to compare the outcomes of FCM (maximum of 2 doses, 500 or 1000 mg iron) and IS (up to 11 infusions, 200 mg iron) treatments in subjects with IDA.

Keywords： iron deficiency     anemia     intravenous iron     ferric carboxymaltose     iron sucrose     Hb response     early response    

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Synergistic effects of sodium hypochlorite disinfection and iron-oxidizing bacteria on early corrosionin cast iron pipes

Frontiers of Environmental Science & Engineering 2022, Volume 16, Issue 6, doi: 10.1007/s11783-021-1506-3

Abstract:

• The early corrosion process in the cast iron pipes was investigated

Keywords： Cast iron pipe corrosion     Drinking water distribution systems     Chlorine disinfection     Iron-oxidizing    

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Ultrasound-assisted co-precipitation synthesis of mesoporous Co3O4–CeO2 composite oxides for highly selective

Frontiers of Chemical Science and Engineering 2022, Volume 16, Issue 8,   Pages 1211-1223 doi: 10.1007/s11705-022-2145-3

Abstract: The one-step highly selective oxidation of cyclohexane into cyclohexanone and cyclohexanol as the essential intermediates of nylon-6 and nylon-66 is considerably challenging. Therefore, an efficient and low-cost catalyst must be urgently developed to improve the efficiency of this process. In this study, a Co3O4–CeO2 composite oxide catalyst was successfully prepared through ultrasound-assisted co-precipitation. This catalyst exhibited a higher selectivity to KA-oil, which was benefited from the synergistic effects between Co3+/Co2+ and Ce4+/Ce3+ redox pairs, than bulk CeO2 and/or Co3O4. Under the optimum reaction conditions, 89.6% selectivity to KA-oil with a cyclohexane conversion of 5.8% was achieved over Co3O4–CeO2. Its catalytic performance remained unchanged after five runs. Using the synergistic effects between the redox pairs of different transition metals, this study provides a feasible strategy to design high-performance catalysts for the selective oxidation of alkanes.

Keywords： Co3O4–CeO2 composite oxides     cyclohexanone     cyclohexanol     ultrasonic-assisted    

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Fluoride ions adsorption from water by CaCO enhanced Mn–Fe mixed metal oxides

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 2,   Pages 236-248 doi: 10.1007/s11705-022-2193-8

Abstract: Novel CaCO3-enhanced Mn–Fe mixed metal oxides (CMFC) were successfully prepared for the firstThese oxides were then employed as an adsorbent for adsorptive removal of excess fluoride ions.

Keywords： mesoporous materials     metal oxides     fluoride ion     adsorption mechanism    

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Application of metal oxides-based nanofluids in PV/T systems: a review

Frontiers in Energy 2022, Volume 16, Issue 3,   Pages 397-428 doi: 10.1007/s11708-021-0758-8

Abstract: Having the wide application of metal oxides in energy technologies, in recent years, many researchersThis paper summarizes recent research activities on various metal oxides (Al2O3

Keywords： metal oxide     nanofluids (NFs)     nanoparticles (NPs)     optical filter     PV/T systems     solar energy    

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Performance of iron-air battery with iron nanoparticle-encapsulated C–N composite electrode

Frontiers in Energy doi: 10.1007/s11708-023-0913-5

Abstract: Highly efficient and stable iron electrodes are of great significant to the development of iron-air batteryIn this paper, iron nanoparticle-encapsulated C–N composite (NanoFe@CN) was synthesized by pyrolysisNeutral K2SO4 electrolyte can effectively suppress the passivation of iron electrodeCompared to the pure nano-iron (NanoFe) battery, the NanoFe@CN battery has a more stable cycling stability

Keywords： energy storage and conversion     metallic composites     nanocomposites     iron-air battery     iron anode    

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Mechanical properties of vanadium-alloyed austempered ductile iron for crankshaft applications

Frontiers of Mechanical Engineering 2023, Volume 18, Issue 3, doi: 10.1007/s11465-023-0746-2

Abstract: This study focused on the development of austempered ductile iron (ADI) with desirable combination of

Keywords： austempered ductile iron (ADI)     vanadium alloying     mechanical properties     crankshafts     retained austenite    

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Crystalline mesoporous transition metal oxides: hard-templating synthesis and application in environmental

Zhen MA, Bei ZHOU, Yu REN

Frontiers of Environmental Science & Engineering 2013, Volume 7, Issue 3,   Pages 341-355 doi: 10.1007/s11783-012-0472-1

Abstract: Although mesoporous metal oxides have lower surface areas compared to mesoporous silicas, they generallyMesoporous metal oxides can be synthesized via a soft-templating or hard-templating approach, and theseIn this review, we summarize the synthesis of mesoporous transition metal oxides using mesoporous silicas

Keywords： mesoporous materials     silica     metal oxide     hard-templating     environmental catalysis    

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Title Author Date Type Operation

Redox reactions of iron and manganese oxides in complex systems

Jianzhi Huang, Huichun Zhang

Journal Article

Modified iron-molybdate catalysts with various metal oxides by a mechanochemical method: enhanced formaldehyde

Xue Liu, Lingtao Kong, Shengtao Xu, Chaofan Liu, Fengyun Ma

Journal Article

Catalytic ozonation performance and surface property of supported Fe

Zhendong YANG, Aihua LV, Yulun NIE, Chun HU

Journal Article

Catalytic combustion of volatile organic compounds using perovskite oxides catalysts—a review

Journal Article

Multivalent manganese oxides with high electrocatalytic activity for oxygen reduction reaction

Xiangfeng Peng, Zhenhai Wang, Zhao Wang, Yunxiang Pan

Journal Article

The role of manganese oxides in the activation of peroxymonosulfate (PMS)

Jianzhi Huang, Huichun Zhang

Journal Article

Review on research and application of mesoporous transitional metal oxides in water treatment

Minghao SUI, Lei SHE

Journal Article

randomized, controlled, open label non-inferiority trial of intravenous ferric carboxymaltose versus ironsucrose in patients with iron deficiency anemia in China

Journal Article

Synergistic effects of sodium hypochlorite disinfection and iron-oxidizing bacteria on early corrosionin cast iron pipes

Journal Article

Ultrasound-assisted co-precipitation synthesis of mesoporous Co3O4–CeO2 composite oxides for highly selective

Journal Article

Fluoride ions adsorption from water by CaCO enhanced Mn–Fe mixed metal oxides

Journal Article

Application of metal oxides-based nanofluids in PV/T systems: a review

Journal Article

Performance of iron-air battery with iron nanoparticle-encapsulated C–N composite electrode

Journal Article

Mechanical properties of vanadium-alloyed austempered ductile iron for crankshaft applications

Journal Article

Crystalline mesoporous transition metal oxides: hard-templating synthesis and application in environmental

Zhen MA, Bei ZHOU, Yu REN

Journal Article